{"created":"2023-05-15T12:22:23.029769+00:00","id":13570,"links":{},"metadata":{"_buckets":{"deposit":"7e86f4db-90c8-4425-ba30-850bf6313a90"},"_deposit":{"created_by":10,"id":"13570","owners":[10],"pid":{"revision_id":0,"type":"depid","value":"13570"},"status":"published"},"_oai":{"id":"oai:kansai-u.repo.nii.ac.jp:00013570","sets":["528:1588:1595:1597","63:71"]},"author_link":["34784","34783","34757","34781","34785","34753","34758","34782","34780"],"item_12_biblio_info_7":{"attribute_name":"書誌情報","attribute_value_mlt":[{"bibliographicIssueDates":{"bibliographicIssueDate":"2019-03-28","bibliographicIssueDateType":"Issued"},"bibliographicIssueNumber":"10","bibliographicVolumeNumber":"11","bibliographic_titles":[{"bibliographic_title":"ChemCatChem"}]}]},"item_12_description_4":{"attribute_name":"概要","attribute_value_mlt":[{"subitem_description":"Ti−Pd alloys were investigated as heterogeneous catalysts for hydrogen autotransfer reactions. This is the first reported study of alloys as catalysts for hydrogen‐borrowing reactions using alcohols. We improved the catalytic activities of alloys by increasing their specific surface areas via a hydrogenation−powdering process. The reactivities and selectivities of hydrogenated Ti−Pd alloys [Ti−Pd (Hy) ] were higher than those of non‐hydrogenated alloy catalysts in N‐alkylation by hydrogen autotransfer using alcohols. A plausible catalytic cycle is proposed based on control studies and deuterium labelling experiments.","subitem_description_type":"Other"}]},"item_12_full_name_3":{"attribute_name":"著者別名","attribute_value_mlt":[{"nameIdentifiers":[{"nameIdentifier":"34783","nameIdentifierScheme":"WEKO"}],"names":[{"name":"近藤, 亮太"}]},{"nameIdentifiers":[{"nameIdentifier":"34784","nameIdentifierScheme":"WEKO"}],"names":[{"name":"竹下, 博之"}]},{"nameIdentifiers":[{"nameIdentifier":"34785","nameIdentifierScheme":"WEKO"}],"names":[{"name":"大洞, 康嗣"}]}]},"item_12_publisher_34":{"attribute_name":"出版者","attribute_value_mlt":[{"subitem_publisher":"Wiley"}]},"item_12_rights_13":{"attribute_name":"権利","attribute_value_mlt":[{"subitem_rights":"This is the peer reviewed version of the following article: Ti−Pd Alloys as Heterogeneous Catalysts for the Hydrogen Autotransfer Reaction and Catalytic Improvement by Hydrogenation Effects, Y. Takahashi, R. Kondo, M. Utsunomiya, T. Suzuki, H. T. Takeshita, Y. Obora, ChemCatChem 2019, 11, 2432., which has been published in final form at https://doi.org/10.1002/cctc.201900318. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions."}]},"item_12_source_id_10":{"attribute_name":"書誌レコードID","attribute_value_mlt":[{"subitem_source_identifier":"AA12433532","subitem_source_identifier_type":"NCID"}]},"item_12_source_id_8":{"attribute_name":"ISSN","attribute_value_mlt":[{"subitem_source_identifier":"18673880","subitem_source_identifier_type":"ISSN"}]},"item_12_version_type_17":{"attribute_name":"著者版フラグ","attribute_value_mlt":[{"subitem_version_resource":"http://purl.org/coar/version/c_ab4af688f83e57aa","subitem_version_type":"AM"}]},"item_creator":{"attribute_name":"著者","attribute_type":"creator","attribute_value_mlt":[{"creatorNames":[{"creatorName":"Takahashi, Yuya"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Kondo, Ryota"}],"nameIdentifiers":[{},{}]},{"creatorNames":[{"creatorName":"Utsunomiya, Masayoshi"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Suzuki, Takeyuki"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Takeshita, Hiroyuki T"}],"nameIdentifiers":[{},{}]},{"creatorNames":[{"creatorName":"Obora, Yasushi"}],"nameIdentifiers":[{},{}]}]},"item_files":{"attribute_name":"ファイル情報","attribute_type":"file","attribute_value_mlt":[{"accessrole":"open_date","date":[{"dateType":"Available","dateValue":"2019-10-08"}],"displaytype":"detail","filename":"KU-0020-20190328-01.pdf","filesize":[{"value":"691.1 kB"}],"format":"application/pdf","licensetype":"license_note","mimetype":"application/pdf","url":{"label":"KU-0020-20190328-01.pdf","url":"https://kansai-u.repo.nii.ac.jp/record/13570/files/KU-0020-20190328-01.pdf"},"version_id":"60375319-1fb8-43d0-9458-8ba94f08ad4f"}]},"item_keyword":{"attribute_name":"キーワード","attribute_value_mlt":[{"subitem_subject":"関西大学","subitem_subject_scheme":"Other"},{"subitem_subject":"Kansai University","subitem_subject_scheme":"Other"},{"subitem_subject":"Alloy catalysts","subitem_subject_scheme":"Other"},{"subitem_subject":"Hydrogen transfer","subitem_subject_scheme":"Other"},{"subitem_subject":"Alkylation","subitem_subject_scheme":"Other"},{"subitem_subject":"Alcohols","subitem_subject_scheme":"Other"},{"subitem_subject":"Heterogeneous catalysis","subitem_subject_scheme":"Other"}]},"item_language":{"attribute_name":"言語","attribute_value_mlt":[{"subitem_language":"eng"}]},"item_resource_type":{"attribute_name":"資源タイプ","attribute_value_mlt":[{"resourcetype":"research report","resourceuri":"http://purl.org/coar/resource_type/c_18ws"}]},"item_title":"Ti–Pd Alloys as Heterogeneous Catalysts for Hydrogen Autotransfer Reaction and Catalytic Improvement by Hydrogenation Effects","item_titles":{"attribute_name":"タイトル","attribute_value_mlt":[{"subitem_title":"Ti–Pd Alloys as Heterogeneous Catalysts for Hydrogen Autotransfer Reaction and Catalytic Improvement by Hydrogenation Effects"}]},"item_type_id":"12","owner":"10","path":["71","1597"],"pubdate":{"attribute_name":"公開日","attribute_value":"2020-03-28"},"publish_date":"2020-03-28","publish_status":"0","recid":"13570","relation_version_is_last":true,"title":["Ti–Pd Alloys as Heterogeneous Catalysts for Hydrogen Autotransfer Reaction and Catalytic Improvement by Hydrogenation Effects"],"weko_creator_id":"10","weko_shared_id":-1},"updated":"2023-05-17T02:21:28.014597+00:00"}